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Sunday, May 5, 2019

GLYCOSIDES PHARMACOLOGY NOTES




1)         Glycyrrhiza:
Synonyms:
Mulethi, Radix glycyrrhizae, Licorice, Jethi Madh, Yashtimadhu
Botanical source:
It consists of subterranean peeled and unpeeled stolons, roots, and subterranean stems of Glycyrrhiza globra Linn.
Family:
Leguminosae
Geographical source:
It is produced in a number of countries like Iran, Russia, Spain, Greece, U.S.S.R., and India.
Cultivation:
It is cultivated by planting rhizomes or stolons cutting in deep, rich, loamy, fertile soil in rows about 4 feet apart in March, addition of farmyard manure has favourable effect on the growth of the plant. Collection of the drug is carried out in autumn in the third or fourth year, by which time extensive development of subterranean part has taken place.
Rhizomes stolons and roots are dug out, buds and rootlets removed, washed, cut into pieces of usually 20 cm length and dried in sun in some cases drug is peeled before drying. Peeled drug is used for direct administration but in preparing for direct administration but in preparing tincture or liquid extracts unpeeled drug is used.
Macroscopical characters:
(i) Condition:
Dry, occurs in the peeled or unpeeled form.
(ii) Shape:
Cylindrical.
(iii) Surface (Outer):
Yellowish brown with longitudinal wrinkles (unpeeled); peeled ones are yellow coloured with fine longitudinal ridges. In case of stolons, scars of the buds can be seen.
(iv) Fracture:
Coarsely fibrous in the bark region and splintery in the wood; fractured surface shows long fibres projecting outwards.
(v) Odour:
Characteristics.
(vi) Taste:
Sweet
Microscopical characters:
1. Periderm: Phellem (cork):
Several layers with tabular cells, outer layers are filled with reddish brown contents and inner few are colourless.
Phellogen: Indistinct Phelloderm: 3-5 layered, immediately below cork, parenchymatous cells whose corners thickened with cellulose (collenchymatous); some cells contain prism of calcium oxalate and minute starch grain.
2. Secondary phloem:
Wide zone with numerous concentrically arranged bundles of phloem fibres each bundle is surrounded by a parenchymatous sheath whose cells contain prisms of calcium oxalate. Radially the fibre bundles alternated with soft phloem elements and tangentially with medullary rays.
3. Medullary rays:
Distinct, bi-to multiseriate, parenchymatous, in continuation with those of xylem however, the rays are narrower in the xylem region and become wider in the phloem region.
4. Secondary xylem:
Well represented, divided (like phloem) by large medullary rays at regular interval. Xylem consists of vessel, fibres and lignified wood parenchyma.
The vessels, fibres and lignified wood parenchyma the vessels, fibres and lignified wood parenchyma the vessels which are relatively wide show scalariform and bordered pitted thickenings.
Wood fibres are also unsheathed by a layer of parenchyma containing crystals. Starch is present in the wood parenchyma.
5. Pith:
Consist of large parenchyma with intercellular spaces and contain few starch grains. Pith absent in root.



Chemical constituents:
1. Saponin glycosides: Glycyrrhizin and glycyrrhetic acid.
2. Flavonoids: Liquiritin, liquiritigenin, isoliquiritin and isoliquiritigenin.
3. Coumarin derivatives: Herniarin, umbelliferone.
4. Bitter principle: glyceramarin.
5. Asparase, β-sitosterol, starch, resin and malic acid

Uses:

1. Demulcent and expectorant.
2. Tonic.
3. Laxative.
4. Diuretic and emollient property.
5. Anti-inflammatory agent.
6. Spasmolytic agent.
7. Cough and peptic ulcer.
8. Chewing gums, chocolate candy, cigarette and chewing tobacco.
Substitutes and Adulterants:
Manchurian Licorice is obtained from Glycyrrhiza uralensis. Colour is chocolate brown and cork exfoliating. Anatomically also it shows peculiarities based on which one can distinguish.
The medullary rays are curved and presence of lacunae can be seen in wood. Being a substitute it does contain glycyrrhizin the active principle but very little of free sugars.
The common adulterant is wild licorice also called Indian licorice, derived from the root of Abrus precatorius (Leguminosae). The root is very toxic due to an alkaloid abrine and therefore should not be used in place of licorice.
The root possesses a peculiar disagreeable Odour and bitter acrid flavour leaving faintly sweet after taste. Microscopically the adulterants are characterized by stone cells.
Powder analysis of liquorices:
1. Organoleptic characters:
(i) Colour: Pale, yellowish- brown.
(ii) Odour: Faint, characteristic.
(iii) Taste: Sweet.
(iv) Odour: Faint, characteristic.
(v) Taste: Sweet.
2. Fibres:
They are yellow coloured fibres in bundles of about 10- 15; the tips of the bundles appear fringed like that of an electric cable.
3. Calcium oxalate:
Parenchymatous sheath of small parenchymatous cell (crystal sheath), each containing a single prism of calcium oxalate, encircle the above fibres; scattered prism are also seen (mostly twin prisms).
4. Wood elements:
vessels large, with numerous bordered pits.
5. Starch granules:
Both simple (oval to elongated) and compound (not many), minute.

2) GINSENG
Synonyms:
            Radix Ginseng, Shin-seng, Panax root, Ginseng root, Korean ginseng, Chinese ginseng and true ginseng.

Description.
Ginseng is the dried root of Panax ginseng (P. schinseng) (Araliaceae) Collected from 5-6 years old plants, in autumn, carefully cleaned and dried. Other varieties of ginseng include Panax quinquefolius (Panax quinquefolium, American Ginseng) and P. pseudoginseng (P. notoginseng, Himalayan ginseng). The root commonly known as Siberian or Russian ginsengbelongs to the same family, Araliaceae, but is an entirely different plant, Eleutherococcus senticosus (Acanthopanax senticosus).Brazilian ginseng is reported to be derived from another unrelated plant, Pfaffia paniculata Martius, family Amaranthaceae (Brazilian ginseng) and Rumex hymenosepalus Torrey, family Polygonaceae (Wild red desert ginseng or American wild red ginseng). Ginseng contains complex mixtures of saponins termed ginsenosides or panaxosides. At least 13 saponins have been isolated from extracts of P. ginseng roots.

Names meaning in English:
Panax derived from the Greek word panacea meaning “all-heal” or “all-cure”. Ginseng, Chinese (Wade-Giles Romanization) Jen Sheng, or (Pinyin) Ren Sheng (root of heaven). Ginseng is derived from the words Jen sheng, which, in addition to 'man-like root'. Chines word xi yang shen means  American Ginseng , Japanese ginseng (chikusetsu ninjin, ninjin means carrot).

     


       

 
Pharmacopoeias.
In Chin., Eur., and Jpn. Also in US (as Asian Ginseng and American Ginseng). US includes additionally powdered forms of these two varieties of ginseng. Jpn also includes Red Ginseng, the dried root of P. ginseng which has been steamed. Chin. and Jpn also include Rhizoma Panacis Japonica from Panax japonicusEur.  also includes Notoginseng Root from P. notoginsengChin. also includes Radix Notoginseng from P. notoginseng, and Rhizoma Panacis Majoris from P. japonicus var. major and P. japonicus var. bipinnatifidus.

Ph. Eur. 6.2 (Ginseng). The whole or cut dried root of Panax ginseng. It contains not less than 0.4% of combined ginsenosides, Rg1 (C42H72O14,2H2O = 837.0) and Rb1(C54H92O23,3H2O = 1163.3), calculated with reference to the dried drug. Protect from light.

USP 31 (Asian Ginseng). The dried roots of Panax ginseng (Araliaceae). It contains not less than 0.2% of ginsenoside Rg1 and not less than 0.1% of ginsenoside Rb1, both calculated on the
dried basis. Store in a dry place at a temperature of 8° to 15°C.

USP 31 (American Ginseng). The dried roots of Panax quinquefolius (Araliaceae). It contains not less than 4.0% of total ginsenosides, calculated on the dried basis. Store in airtight containers. Protect from light and heat.

Ginseng Cultivation:
Most of the drug is collected from plants which are cultivated in various parts of the United States and Canada (American ginseng) and in China, Korea and Japan (Chinese ginseng).The ginseng plant demands a relatively rough climate, though the air temperature throughout the year must remain between 0-25°C. Also, a special type of soil is necessary. The ground temperature must be constant as possible, an artificial fertilizer is never employed but only a fertilizer made of ginseng leaves gathered. The plants do not withstand direct sunlight and must be protected by specially constructed sheds.The plants are propagated from seeds which should be sown in light loam rich in humus and in shade of woodland or orchard, well drained land and some cultivation are necessary for a good crops. 

Ginseng Collection:

The roots are dug from 3 to 6 years old plants in late summer or autumn, washed and carefully dried. Fresh root dug out of the soil is covered with pathogenic germs which remain on it after careful washing. A sterilization process is thus necessary to ensure stability of the roots and to avoid any chance of infection irrespective of whether the root is eaten as such in small slices, as many Asian do, or whether a preparation made from the root is taken.


Ginseng Preparation:
In China, ginseng roots are especially treated by an unknown process which renders them somewhat translucent and horny. Similar results can be obtained by treating the fresh, cleaned roots with recently slaked lime.
White ginseng can also be obtained commercially with the surface “skin” removed by careful peeling. Dried white ginseng, if stored carefully, can retain saleable quality for about 12–15 months. Compared with intact ginseng roots, peeling of ginseng roots resulted in a substantial decrease (approximately 20-30%) in total ginsenoside contents.
 Red ginseng (Korean ginseng) indicates an alternative method of preservation of ginseng. The cleaned roots are sterilised by steam treatment at a temperature of 120° to 130° C for 2 to 4 hours. Sugars present in the roots partially caramelise causing the characteristic red-brown colouration, hence the name “Red Ginseng”. The saponin content of red ginseng is increased during processing. Further observed that in terms of total saponin content the best 6- year old red ginseng came from Korean sources followed by Japanese and Chinese products. The heat treatment increases the hardness of red ginseng roots and also produces chemical artefacts. Carefully stored red ginseng will retain its quality for 2–3 years.
The drug is extensively used in China and it has been estimated that about 300,000 pounds of ginseng are exported annually from the United States. The supplies are not only obtained from wild plants, but also from cultivated plants in various localities in United States and in Asia.

What is G 115 :
G115 being the abbreviation for standardized ginseng extract. It, is a natural product from genuine Panax ginseng. G115 is standardized i.e each dosage unit of G115 contains an accurately determined and equal quantity ofginsenosides.
Morphological Description:
The plant is shrub reaching a height of 60 to 70 cm. The stem carries whirl-fixed, palmate leaves. The fruits are light-red berries about 1 cm. in diameter, containing 1 to 2 flat, white disc­-shaped seeds.
Ginseng root is subcylindrical, somewhat spindle-shaped  fleshy   when dry it is brittle, up to 25 cm long, 0.7 to 2.5 cm in diameter, with 2 to 5 large branches less frequently branched. The body of the root is thickened, almost cylindrical with distinct annulations at top.
The outer surface of root is longitudinally, less frequently spirally wrinkled and exhibiting root scars. On maceration, which goes on slowly, the wrinkles disappear and the surface becomes smooth. In the upper part of the root there is a constricted, transversely wrinkled rhizome, the neck, short with several stem scarsOne or several adventitious roots may emanate from the neck. Rhizomes bear leaf scars the number of which gives an indication of the age of the plant. The external color varying from yellowish white (American and Chinese) to yellowish-brown (Korean); fracture is short and mealy. Ginseng root has a slightly aromatic odor and specific taste which is sweetish, pungent mucilaginous and slightly bitter.
Internally pale yellow to yellowish-brown and exhibiting a broad soft, whitish bark, a dark brown cambium line and a distinctly radiate, hard wood. Scattered through the bark and wood are numerous oil and resin canals which in older roots have a brownish- red  resinous content.

Microscopic differentiation between Panax species
species
Powder
Starch
Calcium oxalate
Panax ginseng (unprocessed ), Panax quinquefolius
Color is beige to white; soft texture
Present
Present
Panax ginseng (processed )
Color is pale to dark reddish brown or pale yellow-brown; hard, more crystallized texture to touch
Absent; transformed into gelatinous mass due to steaming
Present
Panax psudoginseng
Color is beige to yellow
Present and larger than in other Panax species
Infrequent or absent
Constituents:

1- Saponins  termed Ginsenosides by Japanese workers and Panaxosides by Russian workers. However, the two series of compounds do not appear to be absolutely identical with respect of the sugar moieties. Some 13 ginsenosides (e.g. ginsenosides Ro, Ra, Rb1, Rb2, Rc, Rd, Re, Rf, Rg1, Rg2, Rg3, Rhand Rh2.) have been described and designated according to their Rf    values in a particular solvent system. They noted that the protopanaxadiol-derived Rb group (Rb1 and Rb2) and the protopanaxatriolderived Rg group saponins were quantitatively the main glycosides present. The Panaxosides are termed panaxoside A, B, C, etc. The studies of the American chemist E. J. Staba and his colleagues on the indigenous P. quinquefolium revealed that the saponins identified asPanaquilins by earlier workers were also identical with the ginsenosides.
The overall yield of glycosides in Panax ginseng roots varies between 0.5 and 4.0 per cent and is age-dependent. Mild acid hydrolysis of the mixed ginsenosides revealed three principal structural types based on:-
a) the tetracyclic, dammarene, triterpenoid sapogenin (20-S)-protopanaxadiol,
b) the tetracyclic, dammarene, triterpenoid sapogenin (20-S)-protopanaxatriol,
c) the pentacyclic, triterpene oleanolic acid.
On hydrolysis the panaxosides afford principally oleanolic acid, panaxadiol and panaxatriol. The two latter appear to be artefacts arising during hydrolysis. Ginseng root, therefore, contains a mixture of both Tetracyclic and Pentacyclic triterpenoid saponins.
Some of the ginsenosides (Panaquilins) of   Pquinquefolium are the same as those of   the Chinese and Korean drug; others appear to differ.
Correlation of the nomenclature of ginsenosides, panaxosides and panaquilins

Ginsenoside
Panaxoside
Panaquilin
Ro
-
-
Ra
F
-
Rb
E
B
Rc
D
C
-
-
E1
Rd
C
E2
Re
B
E3
Rf
-
-
Rg1
A
G1
Rg2
-
G2

2- High molecular weight polysaccharides (glycans), for P. ginseng these are known as panaxans and they have been shown to have hypoglycaemic activity.
3- Straight-chain acetylenic compoundsEssential oila camphor-like substance named panacene which he had isolated from an extract of the root of the American ginseng P. quinquefolium L.   and Vitamins.
4- Among the nonsaponin constituents of red ginseng was the food flavouring agent 3-hydroxy-2-methyl-pyran-4-one and its glucoside. Such compounds may be artifacts generated during preparation of the red ginseng.

Actions and Uses:

1- As a general tonic and stimulant:
 ginseng can strengthen the debilitated body, for asthenia, stimulating recuperation, improving the quality of life and for sexual impotence.

2- An adaptogen defined in many ways: for different types of stress
A- the ability of ginseng (Panax ginseng), Siberian ginseng (Eleutherococcus spp) and related Araliaceous drugs to increase the nonspecific resistance of the host to several types of stresses.

B- This normalising phenomenon presented by ginseng was referred to as “adaptogenic activity”, a controversial concept. In effect there was a higher state of defence preparation and the adaptogen, which was also known as a non-specific immunomodulator or neuroimmunological regulator.

 C- It is also certain that ginseng is of value in the countering of stresses due to temperature variation, physical strain, disease states and toxic substances.

D- It is a substance that is able to improve the ability of an organism to adapt to differing external or internal disturbances.

E- The enhancement of the body’s non-specific resistance to external stresses or noxious effects of physical, chemical or biological nature.

 3- Nervous system:
A- For all ages as an agent capable of improving memory and intellectual skills.
B- For old age:
I-Protection from neural degeneration, preservation of antioxidant levels and inhibition of malondialdehyde formation collectively retard the inexorable advance of age related deterioration.
II-for the treatment of conditions such as normal ageing, cerebral vascular disease in the aged, senile dementia,Mental function impairment and Alzheimer’s disease.

4- As liver protective agents, in alcohol intoxication therapy.
5- For morphine, cocaine and amphetamine withdrawal problems.
6- Other potential applications of ginseng in anticancer treatment.
7- In preparation for Skin, nail disorders and Hair loss also as Aid to smoking withdrawal.
8- In topical preparations for skin affections such as acne and eczema and in cosmetics still require careful clinical trials to demonstrate indisputably that standardised ginseng phytochemicals or formulations are really effective in human subjects.

Recommended dose
At the practical level, it has been suggested that young and healthy persons should take ginseng in short courses of 2–3 weeks with a two week interval between consecutive courses. The recommended daily dose is 0.5–1.0 g of powdered root or 200 mg of ginseng extract daily divided into two doses, one in the morning two hours before food and one in the evening at least two hours after food.
 It has also been recommended that ginseng should not be taken continuously for periods exceeding three months and others suggest occasional use in treatments comprising a one month course followed by a two months interval before further treatment. Ginseng treatment can be continuous in the aged and the chronically sick.

Precautions
1- Concurrent use of stimulants such as coffee (caffeine) is not encouraged. In the absence of other aetiological factors, it was proposed that prolonged daily use of Siberian ginseng in combination with caffeine and vigorous exercise was responsible for the stroke.
2- Ginseng is not suggested for people with hypoglycemia, high blood pressure, or heart disorders. The ‘ginseng abuse syndrome’ defined as hypertension together with nervousness, sleeplessness, skin eruptions, and morning diarrhoea was experienced by 14 subjects who took ginseng orally in an average daily dose of 3 g for very long period. Abrupt withdrawal precipitated hypotension, weakness, and tremor in 1 user. About 50% of the subjects had stopped the use of ginseng within the 2 years.

Drug interactions
1- Ginseng with phenelzine (MAOI)
 There have been  reports of adverse effects, including headaches, insomnia, tremulousness, and irritability when ginseng was taken with phenelzine.
2- Ginseng with warfarin
 A reduction in the response to warfarin was reported in a patient after taking a ginseng preparation. A study in healthy subjects also found a small reduction in response.
3- Ginseng with digoxin assays
Varieties of ginseng may interfere with plasma-digoxin assays.


Allied species:

1) Eleutherococcus senticosus (Acanthopanax senticosus)
Siberian ginseng, has been employed in the USSR as an abundant and inexpensive substitute for ginseng. It is alsocultivated in China for the roots which are used as a tonic and sedative. ‘' The roots contain active saponiss (eleutherosides), different to those of Panax ginseng, and a series of glucans (eleutherans A-G) and a heteroxylan with adaptogenic properties. In test models the eleutherans have been shown to have hypoglycaemic activity

2) Panax pseudogineseng (Himalayan ginseng).
The roots contain active saponins, Shukla and Thakur have recorded ginsenosides Ro and Rbi, chikusetsusaponin-I Va and other compounds in the Indian root subsp. himalaicus var angustifolius.

3) Japanese ginseng (Panax Japonicum).
It represents the dried rhizomes of Panax repens, a plant growing in Japan and is considered to have properties similar to those of ginseng. The rhizomes  is  horizontal and cylindrical, more or less curved, from 5 to 10 cm, in length and 3 to 6 mm. in thickness. Externally its is yellow-white, nodes considerably thickened and, marked on the upper surface by circular stem-scars The fracture is horny, internally it is whitish marked with small yellowish oil-secretion canals in the cortex, narrow wedges of collateral  vascular bundles separated by broad medullary rays and a large pith. Panax repens contains 20% of saponins, volatile oil and resins. Panax Japonicum and P. japonicumvar. major chikusetsusaponins, ginsenosides and glycans.

4- Indian ginseng (Withania somniferum).
Withania somniferum Dunal is a Solanaceous plant found in southern Europe, India and Africa. It has a reputation in Indian indigenous medicine as a sedative, hypnotic and antiseptic agent. Extracts of the plant demonstrate antimitotic activity. Typically the plant yields tropane alkaloids and steroidal lactones named withanolides but no ginsenosides.

3) Dioscorea

Synonyms:

Yam

Biological source:

Dioscorea consists of the dried tubers of a number of wild and cultivated Dioscorea species like D. deltoidea Wall, D. prazeri Prain, D. floribunda Mart and D. composite.
Family:
Dioscoreaceae

Geographical source:

Dioscorea is found in North America, Japan, China, Mexico, India and Nepal. In India, the plant grows wildly in Western Himalayas, Karnataka, Kashmir, West Bengal, etc.

Macroscopical Characters

1. Rhizomes of D. deltoidea: Horizontal tubers, digitate, chestnut brown with recoiling roots.
2. D. prazeri: Stout horizontal creeping, freely branched, branched about 10 cm long; 1.5 to 2 cm wide, grey brown-blackish, fresh white or creamy.
(i) Odour: Odourless.
(ii) Taste: bitter.

Chemical constituents:

1. Steroidal saponin glycosides: Dioscin and its aglycone is diosgenin. Small quantity of Hecogenin.
2. Resin-Botagenin.
3. Alkaloids: dioscorine.
4. Sterol: Cholesterol, stigmasterol, P-sitosterol.
5. Enzyme: sapogenase.

Uses:

1. Diosgenin is used as a precursor for the synthesis of many steroidal drugs like corticosteroids, sex hormones and oral contraceptives.
2. It is also used in rheumatism.

Allied species:

1. Dioscorea esculenta:
It is a prickly climber; tuber 4 too many stalked, produced in branches close to the surface of the ground. The tubers are starchy and free from dioscorine. They have a sweetish taste; in flavour and mealiness, closely resemble potatoes. The tubers are applied for swelling.
2. Dioscorea. deltoidea:
It is an extensive climber with unarmed stem twining to the left. The tubers are rich in saponin and are used for washing silk, wood and hair, and in dyeing. They kill lice.
3. Dioscorea globra:
It is a climber with stems twining to the right. This species occurs in Assam, Bengal, Bihar, Orissa, and Andaman. The tubers are used as food edible.
4. Dioscorea oppositifolia:
It is a climber with glabrous or finely pubescent stem. The tuber is usually single with few rootlets; skin reddish; flesh white, soft and edible. The tubers are used externally to reduce swellings.
Isolation of diosgenin:
The tubers are washed, dried, sliced and extracted with hot water or 95% ethyl alcohol for several hrs. The alcoholic extract is concentrated under vacuum and the glycosides is precipitated with solvent ether or by lead acetate (in the case of acid saponin) followed by hydrolysis and extracted with petroleum ether, 40-60°C will isolate the diosgenin.


CARDIO-ACTIVITY STEROLS
Digitalis:

Biological source:

Digitalis consists of dried leaves of Digitalis purpurea Linn. After collection leaves are dried immediately at temperature below 60 C and they contain no more than 5% moisture. After drying leaves are stored in moisture proof container.
Family:
Scrophulariaceae

Geographical source:

It is found in European countries, England, France, Germany, North America and India. In India, it is cultivated in Kashmir and Nilgiri Hill.

Cultivation and collection:

It is a biennial or perennial herb. It is about 1 to 2 metres in height. The seed of digitalis are small in size, so they are mixed with sand for sowing. Leaves are collected in both the years but leaves collected when 2/3 of flowers are fully developed. The seedling is than transplanted into the field. Generally the leaves are collected in the early afternoon, with a belief that maximum cardio-active glycosides are present at that time.
The leaves are immediately dried after collection below 60 C and dried leaves are stored in airtight containers. The dried leaves should not contain more than 5% moisture, since it promotes hydrolysis of cardiac glycosides resulting in loss of cardiac activity.

Macroscopical characters:

(i) General appearance: Usually broken and criped.
(ii) Shape: Ovate-lanceolate.
(iii) Size: 10 to 40-cm. Long and 4 to 10 cm.
(iv) Wide Margin: Crenate or dentate
(v) Apex: obtuse or rounded
(vi) Base: Tapering, decurrent
(vii) Upper Surface: Slight pubescent, dark green, little wrinkled, one water pore present near each tooth
(viii) Lower surface: Grayish-green, very pubescent
(ix) Venation: Pinnate, mid-rib, lateral vein, veinlet and still smaller vein lets prominent on the under- surface; lateral vein leaves the mid- rib, at an acute angle and anatomies on the margin.
(x) Petiole: Winged, 2.5 to 10 cm. long
(xi) Odour: Characteristic.
(xii) Taste: Bitter
Digitalis is dorsiventral and can be easily identified due to the presence of characteristic simple covering and glandular trichomes. The covering trichomes are uniseriate; usually three to four cells long, having collapsed cells, acute apex and finely warty cuticle. The glandular trichomes have a short unicellular stalk and bi-cellular or rarely unicellular head. These glandular trichomes are usually located over the veins. Further anomocytic (Ranunculaceous) type of stomata is also present mainly on the lower surface.

Microscopical characters:

1. Lamina:
a. Upper epidermis:
Single layered with more or less rectangular cells having a distinct cuticle. Abundant covering and glandular trichomes emerge from the upper epidermal layer. Covering trichomes are uniseriate, multicellular (3-6 Celled), mostly straight, warty and with blunt tips. Certain cells of the covering trichomes are collapsed, thus forming a diagnostic feature for the identification. Glandular trichomes are with either unicellular or bi-cellular terminal (through rare) stalk having unicellular or bi-cellular terminal gland few stomata are also seen on the upper epidermis.
b. Mesophyll:
It is differentiated into palisade and spongy parenchyma. Calcium oxalate crystals of any type are absent.
c. Palisade:
One layered, compact with radially elongated cells
d. Spongy parenchyma:
4-6 layered and many distinct obliquely cut out veinlet are seen.
e. Lower epidermis:
Similar to upper epidermis and has many stomata and more trichomes compared to those of upper epidermis.
2. Midrib:
The dorsal surface of the midrib is strongly convex and as usual the epidermal layers of lamina continue over the midrib. Below the upper epidermis and above the lower epidermis are seen thin strips of collenchymas. The vascular bundles are surrounded by a distinct endodermal layer, the cells of which contain abundant starch. Within the endodermis, appears a band of the collenchymatous pericycle. Distinct phloem tissue can be seen on the dorsal surface and well developed xylem tissue towards the ventral surface of the midrib.

Chemical constituents:

Digitalis purpurea contains 35 glycosides:
1. The primary glycosides are purpurea glycosides A and B.
2. It also contains Odoroside H, glucogitaloxin.
3. Verodoxin and glucoverodoxin.
4. The digitoxigenin, Digitoxin, Gitoxigenin, gitaloxin are also important medicinal compounds. They are also called secondary glycosides.
5. They contain anthraquinones derivatives like digitolutin, methoxy-2 methyl anthraquinones, etc
6. Contains saponin, flavonoids.
7. Tannins and pectin.

Chemical tests:

1. Raymond’s test:
To the drug, add a few ml of 50% ethanol and 0.1 ml of 1 % solution of m- dinitrobenzene in ethanol. To this solution, add 2-3 drops of 20% sodium hydroxide solution. Violet colours appears, this is due to presence of active methylene group.
2. Legal test:
To the drug, add few ml of pyridine and 2drops of nitroprusside and a drop of 20% sodium hydroxide solution. A deep red colour is produced.
3. Killer killiani test:
Glycoside is dissolved in a mixture of 1 % ferric sulphate solution in (5%) glacial acetic acid. Add one or two drop of concentrated sulphuric acid. A blue colour develops due to the presence of deoxy sugar.
Xanthydrol test:
The crude is heated with 0.1 to 5% solution of Xanthydrol in glacial acetic acid containing 1% hydrochloric acid. A red colour is produced due to the presence of 2-deoxysugar.
4. Baljet test:  Take a piece of lamina or thick section of the leaf and add sodium picrate reagent. If glycoside is present yellow to orange colour will be seen.

Uses:

1. Cardiotonic.
2. Used in various forms like tablets or capsules in the treatment of congestive cardiac failure, atrial flutter, trial fibrillation and peroxymal atrial tachycardia.
3. Diuretic in cardiac edema.

Adulterants:

1. Primrose leaves:
Leaves of Primula vulgaris Huds (Fam: Pimulaceae).
2. Comfrey leaves:
Leaves of Symphytum officinale Linn. (Fam: Boraginaceae).
3. Mullein leaves:
Leaves of Verbascum thapsus Linn. (Fam: Scrophulariaceae).
Powder analysis of Digitalis purpurea:
1. Trichomes:
Both covering and glandular, sometimes in fragments.
2. Covering trichomes:
Multicellular (3-6 celled) with blunt tips and finely warty. Certain cells of the trichomes are often collapsed leaving behind only the cell walls.
3. Glandular trichomes:
They less numerous, with both unicellular and multicellular stalk and a bicellular or multicellular terminal gland.
4. Stomata:
They are anomocytic or Ranunculaceous type.
5. Negative characters:
Absence of calcium oxalate crystal.
6. Organoleptic characters:
Colour:
(i) Pale green powder
(ii) Odour: Slight.
(iii) Taste: Bitter.
2) SQUILL
Synonyms:
Urginea, Jangali pyaj
Biological source:
Indian squill consists of dried slices of bulb Urginea indica Kunth.
Family:
Liliaceae.
Geographical source:
It is found in throughout India including Konkan and Saurastra.
Collection:
The bulb is smaller and is collected after flowering. Dry outer membranous scales are removed and cut into slices and dried.

Macroscopical characters:

i. Size: 1-2 cm length and 5-10 mm breadth.
ii. Shape: Curved, slices separate or 4-8 slices joined to the axis.
iii. Surface: Brittle in dry drug but tough in moist drug.
iv. Colour: Yellow- white.
v. Odour: Slight
vi. Taste: Bitter and acrid.

Microscopical characters:

T.S. section of Squill is shows following tissues:
1. Upper epidermis:
Single layered with a moderately thick cuticle, epidermal cells with thin walls, rounded to polygonal at times axially elongated; no trichomes of any kind.
2. Mesophyll:
They form the bulk and is not differentiated and consists only of thin walled, large, polyhedral, colourless parenchyma with intercellular spaces. Numerous bundled of acicular raphides are seen in the parenchymatous cells of mesophyll, at times still embedded in the mucilaginous sheath. Collateral bundles are seen at regular intervals and have phloem towards upper epidermis and a relatively well developed xylem towards the lower epidermis.
3. Lower epidermis:
Similar to upper epidermis but in addition a few stomata are seen.

Chemical Constituents:

1. Cardiac glycosides: Scillaren A and B
2. Enzymes: Scillarenase
3. Scillaren A is crystalline and responsible for the activity of the drug.

Uses:

It is used as Cardiotonic similar to European scilla. Indian Scilla reportedly contains more Proscillaridin A and exported to Germany.
Powder analysis of Urginea indica (Squill):
1. Acicular raphides:
They are large number of acicular raphides mostly in bundles measuring around 1000 micron in length and around 20 micron in width, scattered all over in parenchyma.
2. Parenchyma:
They are colourless and large parenchymatous tissue containing vascular bundles.
3. Negative characters:
Absence of trichomes abundant starch grains, cluster crystals and prism
4. Organoleptic characters:
(i) Colour: Brownish.
(ii) Odour: Slight.
(iii) Taste: Mucilaginous, bitter and acrid.
5. Chemical test:
(a) Mucilage does not turn pink with Ruthenium red but stains with corallin soda solution.
(b) With Iodine water, mucilage turns reddish purple.
3. Negative characters:
Absence of trichomos, abundant starch grains, cluster crystals and prism.
4. Organoleptic characters:
i. Colour: Brownish.
ii. Odour: Slight.
iii. Taste: Mucilaginous, bitter and acrid.
5. Chemical test:
a. Mucilage does not turn pink with Ruthenium red but stains with corallin soda solution.
b. With Iodine water, mucilage turns reddish purple.


Strophanthus

Synonyms:
Semen strophanthi, Strophanthus Seeds
Botanical Source:
Strophanthus consists of dried ripe seeds of the Strophanthus kombe.
Family:
Apocynaceae

Geographical source:

Wild in the forest of East Africa near lakes of Nyasaland and Tanganyika. Portuguese East Africa at present cultivated in Cameroon.
Collection:
Drug is collected mostly from wild plants and to a small extent from cultivated plants. There are about 32 species of Strophanthus. The plants are large, woody climbers, climbing on the large trees in the forests of Africa. Fruit consists of two divergent follicles, which are dehiscent, and many seeded.
Each follicle is 30 cm. Long, 2.5 cm. Broad, tapering both at the apex and base. Mature and ripe fruits are collected in June- July. After collection Epicarp and flashy mesocarp are removed and seeds separated from yellow-brown leathery endocarp and awns usually separated from. Seeds are washed and washed and dried. The seeds are derived from anatropous ovules.

Macroscopical characters:

(i) Shape: Lanceolate and acuminate.
(ii) Size: 1.3-1.8 cm length and 3-5 cm broad.
(iii) Colour: Silvery grey to yellowish green and pale brown.
(iv) Endosperm: Narrow, oily, white below the seed coat.
(v) Fracture: Short.
(vi) Taste: very bitter.
(vii) Odour: slight, Characteristic.

Uses:

1. In Acute cardiac failure.
2. Hypertensive.
3. Diuretic in cardiac edema.

Chemical Tests:

1. Baljet test, legal test and killer killiani test are giving positive tests similar to digitalis.
2. With 80% H2S04, Strophanthus seeds show green colour.

Allied Drugs:

From the large number of Strophanthus species Strophanthus gratus and Strophanthus sarmentosus are important.
1. Strophanthus gratus seed contain only one crystalline glycoside characterized by define m. p., g-strophanthin or ouabairr. Quabain was first isolated from the wood of an Africa tree Acokanthera quabain (Apocynaceae). As G- strophanthidin is a pure crystalline substance it is used as a standard for biological assay of other cardiac glycosides. Activity of g- strophanthidin is nearly double than kstrophanthidin.
2. Strophcrnthus sarmentosus contains glycoside whose aglycone is sarmentogenin. Sarmentogenin contains an additional OH group at 11 positions. Substances with this chemical structure are suitable for synthesis of cortisone and other steroidal hormones by oxidation.
Substances with this chemical structure are suitable for synthesis of cortisone and other steroidal hormones by oxidation.
ANTHRAQUIIONES
1) Aloe
Synonyms:
Aloe, Ghritkumari, Aliyo (Guj.)
Botanical source:
Aloe is the dried juice collected by incision from the bases of the leaves of various species of aloe.
Family:
Liliaceae

Geographical source:

There are about 160 species of aloe from which the following species are important and utilized for the preparation of aloe.
They are found in the countries mentioned as under:
(1) Aloe perryi: Baker:
This is found in Socotra and Zanzibar Islands and in their neighbouring areas. The aloe obtained from this species is known as Socotrines or Zanzibar aloe.
(2) Aloe vera Linn:
This species is also known as Aloe vulgaris Lamarek, Aloe barbadensis Mil or Aloe officinalis Forskal. This species is a native of North Africa but now cultivated in Aruba Bonaire and to a lesser extent in Curacao in West Indies. The aloe obtained from this species is known as Curacao or Barbados aloe.
(3) Aloe ferox Miller and hybrids of this species with aloe Africana and Aloe spicata:
Cultivation and Collection:
The plant is xerophytes and may be herb, shrub or tree and bears a rosette of leaves, which are thick, fleshy, sessile and spiny. Flowers are red or yellow. For cultivation in West Indies young offsets are planted in the soil after the rainy season in rows situated at a distance of 60cm in the natives collect the second year leaves. Because of the spiny nature of leaves the natives protect their hands and feet, cut the leaves near the base.
Put them into kerosene ting and take them to a central place for the preparation of aloe. Juice of aloe is present in parenchymatous cells of paricycle surrounding which are mucilage cells. On incision of leaves juice exudes from pericyclic cells and mucilage cells exert pressure on pericyclic cells and by single incision juice of the entire leaf in drained out.

Preparation of Aloes:

The method of preparation of aloe is different in West Indies and in South Africa.
(1) Curacao of Barbados Aloe:
In West Indies the cut the leaves are arranged with their cut surface on the inner side, on the slides of V-shaped vessel of about 1 to 1.5 meter long and the flowing juice collected in a tin vessel placed below the V-shape vessel. The juice is transferred to copper evaporating pan and heated carefully till the whole mass acquires semi-solid consistency. It is then cooled slowly and stirred during cooling.
These conditions are favourable for the crystallization or barbaloin and this aloe contained crystal of barbaloin because of the presence of which it becomes opaque and is also known as hepatic or livery aloe. It is packed in gourds and allowed to become more solidified. This aloe is known in commerce as Curacao or Barbados aloe.
(2) Cape Aloe:
In South Africa a shallow circular pit is dug and covered with goat skin or canvas and cut leaves are arranged radially. The juice is collected in canvas or goatskin and transferred to a copper-evaporating pan and heated. It is heated till the juice acquires maximum possible solid consistency. It is then cooled quickly without stirring. These conditions are not favourable for the crystallization of barbaloin and as a result this aloe is transparent, and is known as vitreous or glassy aloe, Cape aloe is prepared in this way.
(3) Socotrine Aloe:
Aloe juice is collected in goat or sheep skin and spontaneous evaporation is allowed for about a month when it becomes viscous pasty mass. Arab traders send this pasty mass to Zanzibar or Bombay from where it is exported to Europe in barrels, tins or leather packing. In European countries it is dried in wooden pans with hot air till moisture is about 10%.
(4) Zanzibar Aloe:
This aloe is considered a type of Socotrines aloe but botanical source is not definite and is prepared similar to Socotrine aloe. It is packed in skins of carnivorous animals. This aloe is also known as monkey skin aloe. Socotrine and Zanzibar aloe are opaque.

Characters

Curacao aloe:
(i) Shape: Opaque
(ii) Colour: yellow-brown to chocolate-brown. Inferior over-heated drug is nearly black.
(iii) Odour: strong odour resembles with Iodoform.
(iv) Taste: Bitter
(v) Fracture: waxy.
Cape aloe:
(i) Glassy
(ii) Colour: Dark chocolate or green-chocolate. Small pieces are reddish- brown or yellow coloured or amber.
(iii) Odour: Characteristic, sour
(iv) Taste: unpleasant and bitter.
(v) Texture: Breaks with a glassy fraction
Socotrine aloe:
(i) Masses of different shapes and sizes.
(ii) Colour: yellow -brown to dark brown and opaque.
(iii) Fracture: Irregular and porous.
(iv) Taste: bitter.
(v) Odour: Unpleasant
Zanzibar aloe:
(i) Opaque, more firm than Socotrine
(ii) Colour: brown.
(iii) Fracture: smooth as wax.
(iv) Odour: considered pleasant
(v) Taste: bitter.

Chemical Constituents:

Aloe may contain upto 30% aloin which is a mixture of three isomers: barbaloin, β-barbaioin and isobarbaloin. Barbaloin present in all the four varieties is slightly yellow-coloured, bitter, water-soluble, crystalline glycoside.
β-barbaloin is amorphous and present in Cape aloe and can be produced from barbaloin on heating. Isobarbaloin is crystalline, present in Curacao aloe and in traces in Cape aloe and absent in Socotrine and Zanzibar aloe and is probably a mixture of barbaloin and polyphenols responsible for its colour tests. Barbaloin is a C-glycoside compared to common O-glycosides.
Aloe also contains aloinsides A and B, O-glycosides of aloin in which L-rhamnose is combined with OH of hydroxymethyl group at 11-.C. atom. Barbaloin on hydrolysis yields aloe emodin anthrone and glucose. Besides aloe-emodin anthrone, aloe-emodin anthranol and aloe-emodin are also present. Aloe contains a resin, which is ester of P.coumaric acid or P. hydroxy cimammic acid esterified with aloeresinotannol.

Chemical Tests:

For carrying out the tests a clear solution of aloe is prepared as follows: Boil 1 gm with 100m] of water, allow it to cool; add 1 gm kieseliguhr, stir, it well and filter through filter paper.
1. Borax test:
Take 10 ml of solution and add 5 gm of borax and heat. Green colour fluorescence is seen which is due to aloe-emodin anthranol. This test becomes more sensitive, if 5 to 10 drops of this reaction mixture are taken a test tube and tilled with water.
2. Bromine Test:
Add equal volume of bromine solution to solution of aloe. Bulky yellow precipitate of tetrabromaloin is formed.
3. Modified Anthraquinones Test:
Take 0.1 gm of drug and add 5ml of 5% solution of ferric chloride and 5ml dilute hydrochloric acid and heat on boiling water-bath for 5 minutes, cool the solution and shake gently with a organic solvent like benzene. Separate the organic solvent layer and add an equal volume of dilute ammonia. A pinkish red colour is formed in ammonical layer. This test is of C. glycoside.
4. Cupraloin Test:
Dilute 10 ml of the solution of aloe to 10 ml with water and add to it 1 drop of copper sulphate solution. Bright yellow colour is produced. Add 10 drops of saturated solution of sodium chloride. Colour change to purplish. Add 20 drops of 90% alcohol, the purplish colour persist.
5. Nitrous acid test:
Add few small crystals of sodium nitrite and few drop of dilute acetic acid to 5 ml of solution of aloe. Pink of purplish colour is produced.
6. Nitric acid Test:
Different aloe show different colours with nitric acid:
(a) Curacao aloe deep reddish -brown
(b) Socotrine aloe – Pale yellow brown
(c) Zanzibar aloe- Yellow -brown
(d) Cape aloe- First brown, changing to green later
Nitric acid test can be performed by taking little Coarse drug on while porcelain tile and adding nitric acid to it

Uses:

1. Aloe and aloin are strong purgative and in higher doses may act as abortifacient.
2. It used alone, aloe causes griping and is usually combined with carminatives or antispasmodic like belladonna or hyocyamus.
3. Ointment of aloe gel is used in sunburns, thermal burns, radiation burns, and abrasion and skin irritation and prevents ulceration and malignancy.

Senna
Synonyms:
Indian Senna
Biological source:
Tinneveley Senna consists of the dried leaflets of Cassia angustifolia Vahl
Family:
Leguminaceae.
Geographical source:

Tinneveley Senna grows in Tirunelveli district and also many parts of South India.
Collection:
Tinnavelley Senna plant is similar to Alexandrian senna plant and is cultivated in South India in areas adjoing Tinnavelley and exported from Tuticorin.
The plant is very sensitive to temperature and if the temperature falls below + 10°C, the plant dies. Because of cultivation, this plant has become very luxuriant. The collection of leaves takes place before flowering season. For collection each leaf is carefully picked from the plant by hand and afterwards they are dried in shade with care. Because of drying in shade, their natural green colour is maintained.
After drying leaves are packed in bales with pressure applied in packing, transverse and oblique impression are found on the leaves. They are less brittle and hence are more or less entire leave. They are less brittle and hence are more or less entire and in good condition.
They were considered better and had good demand and fetched high price but now their price in International market is decreasing because of less percentage of sennosides. Drug collected from dry area is inferior. Every year in India from 5,000 to 7,000 tons of leaves and fruits are obtained by cultivation. Leaves from 67% and fruits form 33% of the drug. However because of probably improvement of quality, price of senna and quantity of export have increased and in 1978- 79, 4782 tons of the drug worth Rs. 20 million were exported.
Microscopical characters:
Upper epidermis:
Single layer with polygonal cells covered on the outer side by a thick warty cuticle. Some epidermal cells contain mucilage. Only covering trichomes emerge from the epidermis layer. Trichomes are non-glandular short, thick, unicellular, non-lignified, warty and curved at the bulbous base. Stomata are seen at regular intervals.
Mesophyll:
It is differentiated into palisade and spongy parenchyma. Being a unifacial or isobilateral leaf; palisade is further differentiated into upper and lower palisade.
Upper palisade:
Single layered, compact with elongated, narrow, columnar cells and this continues also over the midrib region.
Spongy parenchyma:
Thin, narrow, loosely arrange between the upper and lower palisade. Vascular strands are seen very frequently. Few sphaeraphides are also seen in the parenchyma
Lower palisade:
It is restricted, unlike upper palisade, to lamina region only. Cells are smaller than those of upper palisade, loosely arranged and their wall are wavy. Lower epidermis: it is very similar to upper epidermis
Midrib:
It presents a flat ventral surface and convex dorsal surface. The epidermal layers are continuous over the midrib. The cells of the lower epidermis however are small with thick cuticle. The cells of the upper palisade, a tissue that appears below the upper epidermis in the midrib region, are relatively smaller Collateral vascular bundle is prominent occupying the central portion of the midrib. Xylem as usual is towards the ventral surface and phloem towards the dorsal surface. The vascular bundle is covered on both the sides (dorsal and ventral) by patches of sclerenchymatous fibrous.
Characteristics of folia senna is that these fibres are unsheathed by a layer of parenchyma, the individual cells of which contain calcium oxalate prisms. Such fibres with crystal sheath can also be seen, if not frequently, in the lamina region.

Chemical constituents:

1. Senna contains anthraquinones glycoside glycosides as sennosides A, sennosides B, sennosides-C, sennosides D, emodin, chrysophenol, Aloe emodin, rhein.
2. Two naphthalene glycoside, i.e. 6-hydroxy musizin glucoside and Tinnevellin glycoside.
3. It also contains yellow flavinol, colouring matter kaempferol and its glycosides kaempfrin,
4. Sterol and its glucoside.
5. Mucilage, resin and calcium oxalate.

Chemical tests:

Borntranger’s Test:
Powdered leaves of Senna are boiled with dilute sulphuric acid, Filtered and cooled. The filtrate is extracted with chloroform or benzene and dilute ammonia is added to it. The ammonical layer becomes pink to red due to the presence of anthraquinones derivative.

Uses:

1. Used as laxative and cathartic.
2. Senna is mixed with carminative drugs due to its gripping action.
3. Powder senna is mixed with vinegar and applied externally to cure skin diseases.

Powder analysis of Senna:

1. Trichomes:
They are only covering type, short, thick, unicellular, warty and frequently cured near the base.
2. Stomata:
Rubiaceous or paracytic type meaning thereby the two subsidiary cells are parallel to the stomal pore.
3. Calcium oxalate:
They are occurring as cluster crystals in the cells of the mesophyll and as prism in a sheath of the cell around the fibres and as well freely distributed in powder.
4. Epidermis:
With polygonal epidermal cells in surface view
5. Mesophyll:
Fragments of leaf showing isobilateral arrangement
6. Organoleptic characters:
(a) Colour: Greyish- green or yellowish- green powder.
(b) Odour: Faint, characteristic.
(c) Taste: Mucilaginous, slightly bitter.
Allied drugs:
1. Arabian Senna:
This is the wild plant of Cassia angustifolia available in Arabia and is used as substitute.
2. Palthe Senna:
This is the dried plant of Cassia auriculata leaves are used as substitute of senna.
3. Dog Senna:
It is obtained from the leaves of Cassia obovata. The leaves are ovate in shape.

Isolation of sennosides:

Senna leaves are powdered to 20-40 mesh and loaded into vertical/ continuous extractors. Acetone at ambient temperature is circulated through the material to remove adherent impurities of pesticides, and other acetone soluble unwanted material of no therapeutic value.
It is then made free of acetone and extracted with 70% V/V alcohol (ethyl or methyl) preadjusted to pH 3.9 with citric acid at temperature 45-50°C. The extraction is continued till washing show a positive test for anthraquinones glycosides (colour reaction or TLC). After extraction, the marc is desolventised and discarded.
The extracted liquid is filtered and transferred to a tank fitted with stirrer. The pH is adjusted to 6.0-6.2 with lime water. It is then concentrated to a paste of 65-70% total solids in a multiple effect evaporator. The paste is dried in rotary vacuum drier at temperature 50-55°C. The flakes obtained are pulverized to a fine powder. It is then sifted to 80 meshes and packed preferably by vacuum sealing.

Isolation of calcium sennosides:

The senna leaves are powdered to 40 meshes in a pulverize and fine powder is removed by sifting. It is then extracted in vertical extractors place in a row, using 80-90% V/V methanol and adjusted to pH 2.9 with any organic acid as extraction medium.
The solvent is circulated intermittently for 6-8 hrs at 40-45°C. The solvent is then transferred to a storage tank. One more extraction is carried out as above the solvent is collected in the same storage tank. It is then taken to a reactor fitted with stirrer (20-30 rpm) through sparkler filter. The filtered liquid is adjusted to pH 3.7- 3.9 with ammonia.
After adjusted the pH, the liquid is stirred for 30-45 minutes and then allowed to stand for one hour. The precipitate thus formed is removed by filtration and clear liquid is transferred to a tank fitted with stirrer of 90 rpm.
It is made up with methanol so that the final concentration of methanol is reached 80% V/V in solution and filtered. 10% solution of stechiometric amount of calcium chloride in methanol is then added. The content is stirred for 1 hr and then liquor ammonia 30% is added with stirring to pH 6.5-6.8. The stirring is continued until pH is stabilized. It is left for one hr. for complete precipitation of sennosides as calcium salts.
The precipitate is filtered in a drum/leaf filter and washed with chilled methanol till pH of filtrate becomes almost neutral. Final washing with methanol, adjusted at pH 6.5 with ascorbic acid, is given. The precipitate is then quickly dried under vacuum at temperature not more than 50°C till the moisture is reduced to less than 3% in flakes. The flakes are pulverized to fine mesh and packed.

Rhubarb
Synonyms:
Rhizome Rhei, Rhei Radix, Revandchini.
Biological source:
It consists of the peeled dried rhizomes and roots of Rheum palmatum Linn. Rheum officinale and other species of rhubarb, excepting Rheum rhaponticum
Family:
Polygonaceae.
Geographical source:
It is found in China, Tibet, Germany and other Europine countries.
Collection:
The large rhizomes are 6- 10 years old and they grow at an elevation of 3000 to 4000 metres. The rhizomes are dug out in September to October. Then the crown and lateral roots are removed. The outer bark is separated by peeling. The rhizomes are then cut into longitudinal slices and dried in shade.

Macroscopical characters:

(i) General appearance: Rounds, flats or high-dried drug
(ii) Size: Rounds, Flats, Length: 5-12 cm. Up to 15cm; thickness upto 5 cm.
(iii) Diameter: 3 to 5 cm.
(iv) Shape: Cylindrical, conical, Piano- convex Barrel shape
(v) Surface: Smooth, pale brown to reddish and mottled due to reddish- brown network of medullary rays in white parenchyma of phloem or xylem. Abnormal or accessory vascular bundles known as star spots and drying holes are seen. Most of the surface is covered with yellow powder.
(vi) Odour: Characteristic, slightly aromatic.
(vii) Taste: bitter, slight, astringent, gritty.
(viii) Star spot: Within the cambium star spots

Chemical constituents:

1. The anthraquinones are chrysophenol, aloe-emodin, emodin, physcion and rhein anthrones or dianthrones are of chrysophenol, emodin. Aloe- emodin or physcion.
2. Heterodianthrone contains two different molecules of anthrones they are from above anthrone.
3. It also contains astringent substances such as ghicogallin free gallic acid, catechins and epicatechin gallate.
4. It also contains starch and calcium oxalate.

Chemical Tests:

(i) Micro sublimation.
(ii) With ammonia gives pink colour.
(iii) With 5% potassium hydroxide give blood- red colour.

Uses:

(i) Purgative (Large dose).
(ii) Antidiarrhoeal in small dose
1. Calcium oxalate crystal:
They are cluster crystals as big as 100 micron in diameter with well defined and pointed corners many in number and scattered all over.
2. Starch granules:
They are sphaeroidal or angular in shape. Both simple and compound (2-6) and show a distinct central hilum.
3. Wood elements:
The Vessels are very wide, reticulately thickened and do not show any lignin reaction with the usual phloroglucinol + HCl.
4. Chemical test:
Powder on treatment with caustic potash gives blood red colour.
5. Organoleptic characters:
(i) Colour: Yellowish brown to reddish brown.
(ii) Odour: Characteristic, empyreumatic odour.
(iii) Taste: Bitter and astringent.


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